So I don't know about the 5100's, but the standard Shocks & Bilsteins are acting as the extended travel/droop limiters. However there's only about another 1.5" of wheel-travel remaining before everything binds up in a ruin-your-ball-joint and upper-arm-hitting-the-frame way. That works out to be about another 3/4" of shock travel. The twin-beam front suspension is really the way to go if you want to really change the overall travel, otherwise whatever you gain in compression travel is subtracted from droop. The spindle lift kits are still going to have the exact same travel, but you're starting with the CV joints now at a much more extreme angle.
I ended up raising the front about 1.75" by cranking the passenger side key and replacing the driver-side key. Now both adjusters are near their mid-point of travel and the truck sits level side-to-side. I also added about 1" of lift to the rear with extended shackles. The rear still has tons of droop with the standard Bilstein shocks. I will say the ride and handling were greatly improved just with lifting the front end a bit and leveling it side to side (it was off by about 3/4" L-R, now I have it about 1/8" higher on the driver side). The new shocks further improved on the handling and I'll be taking it in for an alignment after I replaced the fixed upper control arm bolts with the new caster/camber bolts.